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1 ingle corner-sharing FeO6 linkages in ferric arsenate.
2 paddy soils, and are structural analogues of arsenate.
3 atoms on the ferric hydroxide and O atoms in arsenate.
4 ion was higher for monothioarsenate than for arsenate.
5 ontributes to the resistance to arsenite and arsenate.
6 arsenate and no detectable covalently bound arsenate.
7 ge were involved in the interaction with the arsenate.
8 as subsequently also microbially oxidized to arsenate.
9 d relatively higher accumulation of PCs than arsenate.
10 phosphate (P(i)), and by the P(i)-surrogate, arsenate.
11 atively low levels of framework phosphate or arsenate.
12 robial transformation of monothioarsenate to arsenate.
13 unts of dimethylarsinate, arsenobetaine, and arsenate.
14 red in roots and shoots of plants exposed to arsenate.
15 and the chemically unstable 2-deoxyribose 1-arsenate.
16 r, ArsR2 binding occurred in the presence of arsenate.
17 eficiencies with high levels of arsenite and arsenate.
18 m aerobic to anaerobic conditions containing arsenate.
19 moderate growth defects, respectively, with arsenate.
20 However, crp was essential for growth on arsenate.
21 3 also eliminated growth on and reduction of arsenate.
22 of the single arsC1 is first used to reduce arsenate.
23 c conditions in the presence of fumarate and arsenate.
24 nearly eliminated growth on and reduction of arsenate.
25 ctivity that was increased 1.6-fold by 10 mm arsenate.
26 ls when cultured in medium containing 2.5 mm arsenate.
27 ate transporter that has a high affinity for arsenate.
28 ere glass, iron (oxyhydr)oxides, and calcium arsenate.
29 ggesting that periphyton is a major sink for arsenate.
30 LODs) of 13 muM for arsenite and 132 muM for arsenate.
31 esting some kind of specific interaction for arsenate.
32 ng a self-powered biosensor for arsenite and arsenate.
33 /mM for arsenite and 0.98 +/- 0.02 mV/mM for arsenate.
34 s kg(-1), primarily as the inorganic species arsenate.
35 oxic conditions and reprecipitation of iron arsenate.
36 lectivity toward arsenite in the presence of arsenate.
37 rapidly by strain MLMS-1 when incubated with arsenate.
38 Sulfide-reacted flocs contained primarily arsenate (47-72%) which preferentially adsorbed to Fe(II
40 t it demycothiolates and reduces a mycothiol arsenate adduct with kinetic properties different from t
41 tion of zinc hydroxide carbonate followed by arsenate adorption onto the precipitate was found to be
43 s and activation barriers for three modes of arsenate adsorption to ferric hydroxides were calculated
44 ting arsenic desorption; they promote As (as arsenate) adsorption to the phyllosilicate clay minerals
46 allele (phyA-t) show increased tolerance to arsenate, although to a lesser degree than the ars4ars5
47 s showed increased tolerance to arsenite and arsenate and a greater capacity for arsenate efflux.
48 High ratios of As(V)/AsSum (total combined arsenate and arsenite concentrations) (0.59-0.78), coupl
49 bed to Fe(III)-(oxyhydr)oxides and that both arsenate and arsenite exclusively formed monodentate-bin
51 and surface polymerization was slowest, was arsenate and arsenite sorption not affected by the prese
52 effect of silicate surface polymerization on arsenate and arsenite sorption was studied by use of hem
56 d As species was generally lower compared to arsenate and arsenite, with the exception of the near in
59 erium, here designated WB3, respires soluble arsenate and couples its reduction to the oxidation of a
61 um aerophilum cultured with oxygen, nitrate, arsenate and ferric iron as terminal electron acceptors
63 this DNA contains only trace amounts of free arsenate and no detectable covalently bound arsenate.
65 , then much of the past century of work with arsenate and phosphate chemistry, as well as much of wha
66 inity of basaluminite and schwertmannite for arsenate and selenate is compared, and the coordination
69 selective procedure for the determination of arsenate and total arsenic in food by electrothermal ato
70 oth structural models, we synthesized ferric arsenates and analyzed their local (<6 A) structure by A
73 PvPht1;3 is induced by Pi deficiency and arsenate, and encodes a phosphate transporter that has a
74 ed the activation barriers for desorption of arsenate, and in complexes with -2 charges, the highest
75 r containing dissolved oxygen (DO), nitrate, arsenate, and sulfate was treated in a fixed-bed bioreac
76 cability for treatment of both arsenites and arsenates, and contrary to all known competitive technol
78 anscriptional regulators were common to only arsenate- and arsenite-sensitive genes, respectively.
80 ray absorption near-edge spectroscopy showed arsenate, arsenite, As-(GS)3, and As-PCs with varying ra
82 , GFAJ-1, has been claimed to be able to use arsenate as a nutrient when phosphate is limiting and to
83 Shewanella sp. strain ANA-3, utilization of arsenate as a terminal electron acceptor is conferred by
84 wo of the cya-like genes could not grow with arsenate as a terminal electron acceptor; exogenous cAMP
86 e best of our knowledge, this is the highest arsenate As(V) adsorption capacity ever reported, much h
94 s present in solution led to the presence of arsenate (As(V)) product adsorbed on goethite and in sol
95 ics approach to investigate the mechanism of arsenate (As(V)) tolerance and accumulation in rice.
96 inorganic As species, arsenite (As(III)) and arsenate (As(V)), and their metabolites, methylarsonate
97 ilized for speciation of arsenite (As(III)), arsenate (As(V)), dimethylarsinic acid (DMA(V)), monomet
102 dependent oxidation of arsenite [As(III)] to arsenate [As(V)] occurring under anoxic conditions.
104 isolate 5508 oxidized arsenite [As(III)] to arsenate [As(V)], reduced As(V) to As(III), and methylat
106 d to investigate the adsorption mechanism of arsenate, As(V), and arsenite, As(III), on MNPs by macro
107 ar algae including inorganic species (mainly arsenate--As(V)), methylated species (mainly dimethylars
108 6 octahedra share corners with four adjacent arsenate (AsO4) tetrahedra in a three-dimensional framew
110 in P. vittata extracts was not inhibited by arsenate at 5 mM or by heating at 100 degrees C for 10 m
111 ess toxic than arsenite, but more toxic than arsenate at concentrations >/=25 muM As, reflected in st
112 e (APSAL) capable of detecting intracellular arsenate at the micromolar level for the first time.
116 micromolar amounts of inorganic phosphate or arsenate but was only slightly inhibited by millimolar c
117 portant role of the PC pathway, not only for arsenate, but also for monothioarsenate detoxification.
118 GFAJ-1, that could grow in medium containing arsenate, but lacking phosphate, and that supposedly cou
121 nent either wooden pallets, chromated copper arsenate (CCA) treated wood, or alkaline copper quaterna
122 ses of the Fe K-edge EXAFS spectra of ferric arsenates complemented by shell fitting confirmed Fe ato
125 , Chen et al. describe a novel mechanism for arsenate detoxification via synergistic interaction of g
128 rs and their metabolites (including dimethyl arsenate (DMA), thio-dimethylarsinoylethanol (thio-DMAE)
131 s grown with limiting phosphate and abundant arsenate does not exhibit the spontaneous hydrolysis exp
137 chanisms attributing the enhanced removal of arsenate from solution in the presence of Zn(II) to addi
139 dase had its structure solved and the first "arsenate gene island" identified, provided a draft genom
140 ), i.e., the inorganic arsenite iAs(III) and arsenate iAs(V), and the methylated methylarsonate (MA),
141 entation of cymA in trans restored growth on arsenate in DeltacymA strains of both CN-32 and ANA-3.
142 ty ratio of 8.21, and using the detection of arsenate in drinking water as a model system, we have ac
144 be a remarkable microbe for which there was "arsenate in macromolecules that normally contain phospha
146 tionation of inorganic arsenic (arsenite and arsenate) in environmental solids in combination with it
147 compared it to the sorption of arsenite and arsenate, in suspensions containing 2-line ferrihydrite,
156 ion interaction model similar to the BLM for arsenate is possible, potentially improving current risk
158 tammetric technique, arsenite is oxidized to arsenate leading to its quantitative determination witho
159 ganic arsenite (iAs3+, </= 5 muM), inorganic arsenate (</= 20 muM), trivalent monomethylated arsenic
163 se = 3), based on peak height, for arsenite, arsenate, MMA, and DMA are 0.4, 0.2, 0.5, and 0.3 microg
164 A): TUA1 was defined as the sum of arsenite, arsenate, monomethylarsonic acid, and dimethylarsinic ac
165 lytic base responsible for activation of the arsenate nucleophile and stabilization of the thymine le
166 IR spectroscopy showed that no adsorption of arsenate on a ferrihydrite film occurred at pD 8 in the
167 ere was the most probable type of ligand for arsenate on both phases and for selenate on schwertmanni
171 induced in Arabidopsis seedlings exposed to Arsenate or Cu(2+) , which induces oxidative stress (iii
174 itro groups of Nit(V), forming p-aminophenyl arsenate (p-arsanilic acid or p-AsA(V)), and Rox(III), f
175 as oxo-anions (e.g., perchlorate, chromate, arsenate, pertechnetate, etc.) or organic anions (e.g.,
177 esponsive transcription factor that mediates arsenate/phosphate transporter gene expression and restr
178 sposon burst in plants, in coordination with arsenate/phosphate transporter repression, which immedia
179 ies of inorganic oxoanions such as arsenite, arsenate, phosphite, phosphate, and borate is described.
183 ocal structure of short-range ordered ferric arsenates provides a plausible explanation for their rap
184 eport the first isolation of a dissimilatory arsenate reducer from sediments of the Bengal Basin in W
185 results indicated colocation of sulfate- and arsenate-reducing activities, in the presence of iron(II
187 of 20 min each, DO-, nitrate-, sulfate-, and arsenate-reducing TEAP zones were located within reactor
189 ent combinations of gene knockout, including arsenate reductase (HAC1), gamma-glutamyl-cysteine synth
190 r1105 protein (mw 14.8 kDa) possessed strong arsenate reductase (Km 16.0 +/- 1.2 mM and Vmax 5.6 +/-
191 AW3110), a deletion of the gene for the ArsC arsenate reductase (strain WC3110), and a strain in whic
193 ytic domains exhibited phosphatase activity, arsenate reductase activity was observed only with Cdc25
195 5 of Anabaena sp. PCC7120 which functions as arsenate reductase and phosphatase and offers tolerance
196 1105 of Anabaena sp. PCC7120 functions as an arsenate reductase and possess novel properties differen
197 ion in Escherichia coli lacking a functional arsenate reductase confirmed the arsenate reductase acti
198 irmed the previous observation that the ACR2 arsenate reductase in A. thaliana plays no detectable ro
199 lr1105 enhanced the arsenic tolerance in the arsenate reductase mutant E. coli WC3110 (arsC) and rend
200 bidopsis thaliana allowed us to identify the arsenate reductase required for this reduction, which we
201 sequence and functional similarity with the arsenate reductase ScACR2 from Saccharomyces cerevisiae,
202 uromonas genus and possesses a dissimilatory arsenate reductase that was identified using degenerate
204 r enzyme LmACR2 is both a phosphatase and an arsenate reductase, and its structure bears similarity t
206 umber of eukaryotic enzymes that function as arsenate reductases are homologues of the catalytic doma
207 olutionary viewpoint, LmACR2 and the related arsenate reductases form, together with the known Cdc25
212 Known mechanisms include arsenite efflux, arsenate reduction followed by arsenite efflux and arsen
214 iring chemoautotroph which grows by coupling arsenate reduction to arsenite with the oxidation of sul
215 eriments indicated that Zn(II) increased the arsenate removal from a solution by ferrihydrite at pH 8
216 d to be a plausible mechanism explaining the arsenate removal from a solution in the presence of Zn(I
217 We report the first example of arsenite and arsenate removal from water by incorporation of arsenic
218 he kinetics and efficiencies of arsenite and arsenate removal from water were evaluated using polyalu
220 Two mutants of strain G20 with defects in arsenate resistance were generated by nitrosoguanidine m
221 ne or the arsRBCC operon displayed wild-type arsenate resistance, indicating that the two arsC genes
224 netic analysis demonstrated that spontaneous arsenate-resistant mutants derived from CuR1 all underwe
225 nate sensitivity and 20 human orthologues to arsenate-resistant proteins, including MSH3, COX10, GCSH
226 4-fold reduction in the MICs of arsenite and arsenate, respectively, and complementation of the arsB
234 activity of the Shewanella sp. strain ANA-3 arsenate respiratory reductase (ARR), the key enzyme inv
235 d for this arsenic-based metabolism: (i) the arsenate respiratory reductase (ArrA) and (ii) arsenite
237 num-containing oxidoreductases: specifically arsenate respiratory reductase, ArrA, and arsenite oxida
240 epression system are essential to regulating arsenate respiratory reduction in Shewanella sp. strain
241 family protein, called ArsR2, regulates the arsenate respiratory reduction pathway in response to el
242 coupled to autotrophic arsenite oxidation or arsenate respiratory reduction, occurs only in the proka
243 the metabolically active bacteria, including arsenate-respiring bacteria, were determined by DNA stab
244 Strain MLMS-1 is the first reported obligate arsenate-respiring chemoautotroph which grows by couplin
245 n the enrichment of sequences related to the arsenate-respiring Sulfurospirillum spp. (13) C-acetate
252 lutions did not show a competitive effect on arsenate sorption capacity but had a strong impact on se
255 nation number of 1.6 implied that two uranyl arsenate species with U:As ratios of 1:1 and 1:2 formed
256 time-dependent sorption of two S-substituted arsenate species, mono- and tetrathioarsenate, and compa
258 ility of single species standardization with arsenate standard for accurate quantification of all oth
261 cipitates indicated that precipitates in the arsenate system had the highest water content and that o
262 calcite precipitates revealed only isolated arsenate tetrahedra with no evidence for surface adsorpt
263 ed sulfide oxidation coupled to reduction of arsenate to arsenite could simply enhance abiotic desulf
267 erves as the electron donor for reduction of arsenate to arsenite; and d) As has a high affinity for
269 that Cdc25B and -C may adventitiously reduce arsenate to the more toxic arsenite and may also provide
270 mined the role of phytase and phosphatase in arsenate tolerance and phosphorus (P) acquisition in the
272 ene, for phosphate fertilizer responsiveness/arsenate tolerance in wild grass Holcus lanatus genotype
276 raction of soil pore-water constituents with arsenate toxicity was investigated in cucumber (Cucumis
278 National Park, trithioarsenate transforms to arsenate under increasingly oxidizing conditions along t
279 dependent signaling mechanism that modulates arsenate uptake and transposon expression, providing a c
280 vPht1;3 probably contributes to the enhanced arsenate uptake capacity and affinity exhibited by P. vi
281 range of 1 to 10, and achieves a remarkable arsenate uptake capacity of 303 mg/g at the optimal pH,
284 ides during combined microbial iron(III) and arsenate(V) reduction is thought to be the main mechanis
285 oxides in phosphate-containing growth media, arsenate(V) was immobilized by the newly forming seconda
286 tudy we observed that during bioreduction of arsenate(V)-bearing biogenic iron(III) (oxyhydr)oxides i
287 ization were strongly correlated to measured arsenate values in pore-water (R(2) = 0.76, P < 0.001).
288 The CuO-NP were regenerated by desorbing arsenate via increasing pH above the zero point of charg
289 ioluminescence as a response to arsenite and arsenate was applied during a field campaign in six vill
290 n mechanism for removal of selenate, whereas arsenate was removed by a combination of surface complex
292 1:1 and the 1:2 species, that the bidentate arsenates were bound to uranium with one of the binding
293 and F1 generations accumulated arsenite and arsenate when F0 L4 larvae were exposed to arsenite for
294 ge kinetics of FeFbpA-SO4 with phosphate and arsenate, where first-order kinetics with respect to FeF
295 l cyanide m-chlorophenylhydrazone and sodium arsenate, which are capable of depleting cellular ATP le
296 e prevalent form of arsenic in most soils is arsenate, which is a phosphate analog and a substrate fo
297 e most prevalent chemical form of arsenic is arsenate, whose similarity to phosphate renders it easil
299 Angelellite (Fe4As2O11), a triclinic iron arsenate with structural relations to hematite, can epit
300 anation for the reported growth of GFAJ-1 in arsenate without invoking replacement of phosphorus by a
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