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1 solution multidimensional single- and double-quantum (1)H solid-state NMR spectroscopy with density f
7 cent progress in topological insulators, the quantum anomalous Hall effect, chiral topological superc
8 rana fermion modes in the hybrid system of a quantum anomalous Hall insulator thin film coupled with
9 and the spin dynamics of potential molecular quantum bits, and enriches the guidelines to design mole
10 FTIR/smog chamber experiments and ab initio quantum calculations were performed to investigate the a
14 coined "pseudolaratriene." Combined NMR and quantum chemical analysis verified the structure of pseu
16 Our experimental findings are supported by quantum chemical calculations and noncovalent interactio
17 stry in Li-S batteries through sophisticated quantum chemical calculations, in combination with (7) L
20 approach is presented that combines accurate quantum chemical descriptions with state-of-the-art mode
23 w well-established concepts in the fields of quantum chemistry and material sciences have to be adapt
25 nd K-edge absorption spectroscopy as well as quantum chemistry to determine molecular and electronic
27 mes, such as those that use high-dimensional quantum codes in a modular architecture, have potential
31 rovide evidence of any long-lived electronic quantum coherence, but confirm the orthodox view of rapi
33 tical task for spatial-mode multiplexing and quantum communication - basis-specific principles are in
37 ardware size and reliability requirements of quantum computing algorithms and the physical machines f
38 antum states are most promising for building quantum computing and information storage devices, as th
40 se of molecular electron spins as qubits for quantum computing will depend on the ability to produce
41 l for achieving fidelity in spectroscopy and quantum computing, but inherent nonlinearities and param
42 Given the stringent resource constraints in quantum computing, information passed between layers of
44 ment of layered Sr2 IrO4 induces distinct 1D quantum-confined electronic states, as observed from opt
45 rned by changes in the band structure due to quantum confinement and are most profound if the underly
48 effects of the spatial nonuniform collective quantum confinement of sp(2) domains, and the trapping o
49 que one-dimensional structure enables strong quantum confinement with the formation of self-trapped e
51 ctance mapping", which allows us to suppress quantum corrections to reveal the underlying mechanisms
52 ment swapping may be used to generate remote quantum correlations between particles that have not int
55 al form, enabling DFET to study the stronger quantum couplings between covalently bonded subsystems.
60 energy above twice band gap could indicate a quantum cutting due to the low dimensionality.Understand
61 Via photophysical studies Ni et al. observe 'quantum cutting' in 0D metal-organic hybrid materials ba
63 rting number of 2000 atoms, 1400 atoms reach quantum degeneracy in 300 milliseconds, as confirmed by
64 genides are characterized by valley and spin quantum degrees of freedom, making it possible to explor
66 challenge is to achieve a fully programmable quantum device featuring coherent adiabatic quantum dyna
68 e for generic bottom-up synthesis of complex quantum devices with a special focus on nanowire network
73 interacting system of phonons as well as the quantum discord between distinct degrees of freedoms can
74 ear connection between the amplification and quantum discord like measurements as well as classical c
77 resent study reports the fabrication of CdSe quantum dot (QD)-sensitized photocathodes on NiO-coated
78 t-free, top-down method to create large-area quantum dot arrays with nanometer-scale spatial density
87 s, such as Ti-Si molecular sieves and carbon quantum dots (CQDs), are also briefly appraised in view
90 125 (CA 125) using polyamidoamine dendrimer-quantum dots (PAMAM-QDs) and PAMAM-sulfanilic acid-Ru(bp
94 ned FRET pair, including the donor, CdSe/ZnS quantum dots (QDs), and the acceptor, dextran-binding ma
95 esting nanomaterials, such as semiconducting quantum dots (QDs), metal nanoparticles, semiconductor-m
101 nterface between Si3N4 waveguides and single-quantum dots in GaAs geometries, with performance approa
102 We anticipate that the approach of screening quantum dots not only based on their optical properties,
104 nometer-scale spatial density that allow the quantum dots to interfere with each other and create art
105 sts ranging from classical dyes to drugs and quantum dots, allowing changes in the photochemical beha
106 integrated with proteins, fluorescent dyes, quantum dots, and magnetic nanoparticles can be further
108 based on parametric downconversion sources, quantum dots, colour centres or atoms are fundamentally
109 anic fluorescent dyes ( approximately 4 nm), quantum dots, either small ( approximately 10 nm diamete
110 cavities containing self-assembled InAs/GaAs quantum dots-a mature class of solid-state quantum emitt
121 lay between energetic, entropic, and nuclear quantum effects on the evolution of water clusters from
123 white-light emissions with photoluminescence quantum efficiencies of approximately 20% for the bulk s
124 (EL) peak at 325 nm and achieved an external quantum efficiency (EQE) of about 0.03%, for a deep UV-L
125 Clear improvements in measured detective quantum efficiency and combined energy resolution/energy
126 he great potential of improving the internal quantum efficiency for mid- and deep-UV device applicati
127 larify the necessary means to achieve device quantum efficiency higher than the state-of-the-art GaN:
128 om cut-off wavelength at 77 K and exhibits a quantum efficiency of 31% for a 2 microm-thick absorptio
129 on-optimized NYS:0.10Sm(3+) exhibited a high quantum efficiency of 73.2%, and its luminescence intens
133 ons, as described in the framework of cavity quantum electrodynamics, leads to the hybridization of l
135 Our first three-dimensional simulation with quantum-electrodynamics incorporated shows that a GeV po
137 ing into account the substantial overhead of quantum error correction, and the need to compile into d
143 via the observation of an ambipolar surface quantum Hall effect and quantum oscillations in the Seeb
144 Consequently, the relationship between the quantum Hall effect and topological bulk insulator break
145 ntional two-dimensional systems, this unique quantum Hall effect may be related to the quantized vers
146 gnetic materials and more recently using the quantum Hall effect, parametric permittivity modulation
148 In addition, during the whole procedure, quantum information is almost fully transferred between
149 coupled mechanical resonators are useful for quantum information processing and fundamental tests of
153 can also enable the assembly of large scale quantum information systems and open up new avenues for
155 ide heterostructure LaAlO3 /SrTiO3 , exhibit quantum interference signatures up to room temperature.
157 d in experimental quantum networking, future quantum Internet, and long-distance quantum communicatio
158 diamond, we experimentally demonstrate that quantum interpolation can achieve spectroscopy of classi
162 erization of electroluminescence emitters as quantum light sources, which can be studied with high ti
168 ing this quantum regime entails, inter alia, quantum measurement backaction exceeding thermal forces
171 tope effect (BIE) measurements combined with quantum mechanical (QM) calculations to solve the transi
172 yd for the first time, and two complementary quantum mechanical approaches (CASPT2/MM and PCM/TD-CAM-
173 ng nanosecond time-resolved spectroscopy and quantum mechanical calculations (TD-DFT), it focuses on
175 simulations, thermodynamic integration, and quantum mechanical calculations on aromatic model system
178 ucture and conformational, as well as purely quantum mechanical effects like charge-transfer or excit
180 etics do not follow these predictions unless quantum mechanical tunneling along the heme doming coord
181 thods reviewed here include multidimensional quantum mechanical tunneling, multistructural VTST (MS-V
182 e, we performed electrochemical analysis and quantum-mechanical calculations to describe the mechanis
183 and reveal detailed information on the pure quantum-mechanical contribution to the stereodynamics.
184 classical molecular dynamics simulations and quantum-mechanical density functional theory calculation
186 n 1929, only three years after the advent of quantum mechanics, von Neumann and Wigner showed that Sc
187 rising and counter-intuitive consequences of quantum mechanics, with potent applications in cryptogra
191 use classical molecular dynamics and hybrid quantum mechanics/molecular mechanics calculations at th
192 t between millions of atoms in a solid-state quantum memory prepared by the heralded absorption of a
193 riment that realizes a multiplexed DLCZ-type quantum memory with 225 individually accessible memory c
195 the condensed phase with both classical and quantum methods using explicitly and implicitly solvated
197 We perform here large-scale classical and quantum molecular simulations to study the function of t
199 aterial sciences have to be adapted when the quantum nature of light becomes important in correlated
200 e, we introduce and experimentally realise a quantum network architecture, where the nodes are fully
201 assess nonclassical correlations in an open quantum network, such as quantum transport through nano-
202 The results can be applied in experimental quantum networking, future quantum Internet, and long-di
204 rely on efficient interfacing of dissimilar quantum nodes, as elements based on parametric downconve
206 e on (or 'propensity rule' for) the magnetic quantum number m of the molecules, and a previously unre
210 s are one of the most distinctive aspects of quantum optics, being the trigger of multiple nonclassic
212 an ambipolar surface quantum Hall effect and quantum oscillations in the Seebeck and Nernst effect.
213 ere, the authors provide evidence for such a quantum phase transition in the attractive Coulomb poten
216 scovering pathways to experimentally realize quantum phases of matter and exert control over their pr
218 orbital interaction (SOI) can induce unique quantum phenomena such as topological insulators, the Ra
223 Our experiment offers a novel macroscopic quantum platform to explore the non-Hermitian physics of
226 t connectivity is an important property of a quantum processor, with an ideal processor having random
231 interacted; this is the core ingredient of a quantum repeater, akin to repeaters in optical fibre net
233 tiveness of our proposal by characterizing a quantum resource engineered combining two-photon hyperen
234 coordinate VTST (VRC-VTST), system-specific quantum Rice-Ramsperger-Kassel theory (SS-QRRK) for pred
236 t integrates a nitrogen-vacancy (NV) diamond quantum sensor with optical and microwave waveguide deli
239 alues p approximately 12.7 obtained by dimer quantum simulations are preferred for the argon gas whil
241 loring many-body phenomena on a programmable quantum simulator and could enable realizations of new q
244 earning explores how to devise and implement quantum software that could enable machine learning that
245 of classical magnetic fields and individual quantum spins with orders of magnitude finer frequency r
246 Topological nodal line semimetals, a novel quantum state of materials, possess topologically nontri
250 onsequence of interference between different quantum states has great importance in the fields of chi
252 entanglement, the ability to transport such quantum states robustly over long distances remains chal
254 st apply atomistic simulation techniques and quantum/statistical mechanics methods to understand how
255 cules, and a previously unrecognized type of quantum stereodynamics that has no classical analogue or
256 he continuous scale symmetry of a scale-free quantum system is broken into a discrete scale symmetry
258 ezed light is a key resource in the field of quantum technologies and has already improved sensing ca
261 nowledge gap by obtaining reliable values by quantum theoretical calculations using G4 model chemistr
262 Here we experimentally probe hyper-complex quantum theories, studying one of their deviations from
263 ensity functional theory (DFT), supported by quantum theory of atoms in molecules and natural bond or
266 arises whether there are instances where the quantum time evolution of a macroscopic system is qualit
268 s by employing the donor-bound electron as a quantum transducer, much in the spirit of recent works w
270 We argue that theoretical approaches of the quantum transport community (and in particular, the Gree
272 elations in an open quantum network, such as quantum transport through nano-structures or excitation
275 ction-centered interpretations: instead of a quantum wave passing through both slits, we have a local
276 at harnessing the complex interplay between quantum wavefunctions and various factors such as dimens
277 rent injection efficiency model for a GaN:Eu quantum well (QW) has been developed to clarify the nece
279 tonic insulator gap in an inverted InAs/GaSb quantum-well system at low temperatures and low electron
280 surfaces, wherein distributed semiconducting quantum wells display extreme absorption and emission po
281 tudy a cavity device with four embedded GaAs quantum wells hosting excitons that are spectrally match
282 en-Popper perovskites are solution-processed quantum wells wherein the band gap can be tuned by varyi
283 shba spin-orbit coupling in In0.75 Ga0.25 As quantum wells, which indeed can be tuned by the indium c
285 /g-C3 N4 PHJ, achieving an enhanced apparent quantum yield (AQY) of 27% at 440 nm over PCzF/g-C3 N4 .
286 The abrupt increase in photoluminescence quantum yield at excitation energy above twice band gap
287 n, easily observable even by naked eye, with quantum yield higher than the standard 9,10-diphenylanth
289 cture, a 1.6-fold enhanced photoluminescence quantum yield, and a longer emission lifetime than the s
293 equently, externally measured effective PSII quantum yields may be composed of signals derived from c
297 ll increase both the up- and down-conversion quantum yields, potentially exceeding the Shockley-Queis
298 derivatives with higher intersystem crossing quantum yields, which can be promoted by core heavy atom
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